The look on Sam's face when Gollum calls him a "stupid fat Hobbit" in the second Lord Of The Rings film.
Keeping up with that moment, the "PO-TA-TOES" quote from Sam is also a quite funny line, even his comments afterwards "Boil em, smash em, stick em in a stew."
Other than that, in Pulp Fiction, when they attempt to inject Mia with adraline after a overdose, then her reaction when they stab it into her breast-plate.
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